Structural correlations in diffusiophoretic colloidal mixtures with nonreciprocal interactions

Nonreciprocal effective interaction forces can occur between mesoscopic particles in colloidal suspensions that are driven out of equilibrium. These forces violate Newton’s third law actio  =  reactio on coarse-grained length and time scales. Here we explore the statistical mechanics of Brownian particles with nonreciprocal effective interactions. Our model system is a binary fluid mixture of spherically symmetric, diffusiophoretic mesoscopic particles, and we focus on the time-averaged particle pair- and triplet-correlation functions. Based on the many-body Smoluchowski equation we develop a microscopic statistical theory for the particle correlations and test it by computer simulations. For model systems in two and three spatial dimensions, we show that nonreciprocity induces distinct nonequilibrium pair correlations. Our predictions can be tested in experiments with chemotactic colloidal suspensions.

• Publication year

  2015

• Venue

  Journal of Physics: Condensed Matter

• Publication date

  2015-10-07

• Fields of study

  Medicine, Physics

• Identifiers
  DOI 10.1088/0953-8984/28/2/025102arXiv 1510.01870PMID 26658255
• External record

  Open on Semantic Scholar

• Source metadata

  Semantic Scholar, PubMed

• No claims are published for this paper.

• No concepts are published for this paper.

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