Effect of dissolved organic matter fractions on photodegradation of phenanthrene in ice.

The effect of dissolved organic matter (DOM) fractions on photodegradation of phenanthrene (PHE) in ice was investigated. DOM in surface water and wastewater samples was fractionated using XAD-8/XAD-4 resins into five fractions: hydrophobic acid (HPO-A), hydrophobic neutral (HPO-N), transphilic acid (TPI-A), transphilic neutral (TPI-N) and hydrophilic fraction (HPI). The photodegradation rate of PHE in ice was about 40% greater than that in water. The screening effect and quenching effect contributed 3-12% and 88-97% toward the inhibition of DOM fractions on PHE photodegradation in ice, respectively. The contribution ratios of singlet oxygen (1O2) and hydroxyl radical (OH) produced from DOM fractions to PHE photodegradation rates in ice were 9-31% and 2-13%, respectively. Among five DOM fractions, HPO-A was most efficient in advancing PHE photodegradation in ice through 1O2 mechanism. When excluding the photosensitized effect of 1O2 and OH produced from DOM fractions, the quencing effect of DOM fractions on PHE photodegradation in ice was closely related to their PHE binding ability.

• Publication year

  2019

• Venue

  Journal of Hazardous Materials

• Publication date

  2019-01-01

• Fields of study

  Medicine, Chemistry, Environmental Science

• Identifiers
  DOI 10.1016/j.jhazmat.2018.08.072PMID 30176413
• External record

  Open on Semantic Scholar

• Source metadata

  Semantic Scholar, PubMed

• No claims are published for this paper.

• No concepts are published for this paper.

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