Sulfide‐Based Solid‐State Electrolytes: Synthesis, Stability, and Potential for All‐Solid‐State Batteries

Due to their high ionic conductivity and adeciduate mechanical features for lamination, sulfide composites have received increasing attention as solid electrolyte in all‐solid‐state batteries. Their smaller electronegativity and binding energy to Li ions and bigger atomic radius provide high ionic conductivity and make them attractive for practical applications. In recent years, noticeable efforts have been made to develop high‐performance sulfide solid‐state electrolytes. However, sulfide solid‐state electrolytes still face numerous challenges including: 1) the need for a higher stability voltage window, 2) a better electrode–electrolyte interface and air stability, and 3) a cost‐effective approach for large‐scale manufacturing. Herein, a comprehensive update on the properties (structural and chemical), synthesis of sulfide solid‐state electrolytes, and the development of sulfide‐based all‐solid‐state batteries is provided, including electrochemical and chemical stability, interface stabilization, and their applications in high performance and safe energy storage.

• Publication year

  2019

• Venue

  Advances in Materials

• Publication date

  2019-08-22

• Fields of study

  Medicine, Materials Science, Chemistry, Engineering

• Identifiers
  DOI 10.1002/adma.201901131PMID 31441140
• External record

  Open on Semantic Scholar

• Source metadata

  Semantic Scholar, PubMed

• No claims are published for this paper.

• No concepts are published for this paper.

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