Green Synthesis of Nano-Zero-Valent Iron Using Ricinus Communis Seeds Extract: Characterization and Application in the Treatment of Methylene Blue-Polluted Water

Ahmed M. Abdelfatah,M. Fawzy,Abdelazeem S. Eltaweil,Mohamed E. El‐Khouly

Published 2021 in ACS Omega

ABSTRACT

In this study, the removal of methylene blue dye (MB) from aqueous solution was examined using a novel green adsorbent to overcome the obstacles encountered in chemical methods. Ricinus communis (RC) aqueous seeds extract was herein used as a reducing and capping agent to synthesize a novel nano-zero-valent iron (RC-nZVI) for the adsorption of harmful MB. Structural and morphological characterization of the synthesized RC-nZVI were performed using several techniques, e.g., steady-state absorption, scanning electron microscopy (SEM), transmission electron microscopy (TEM), Fourier transform infrared (FT-IR), energy-dispersive X-ray spectroscopy (EDS), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), and zeta potential. The maximum efficiency of the removal was 96.8% at pH 6 and 25 °C. According to the kinetics study results, the adsorption process obeys the pseudo-first-order model. The experimental equilibrium data were fitted to the Freundlich isotherm model, the maximum adsorption capacity reached was 61.37 mg·g–1, and the equilibrium parameters were determined. The synthesized RC-nZVI possesses good reusability and can be considered as a potential economic and environmentally friendly adsorbent.

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